Couldn't let some of these go, I'm a huge softie when it comes to nostalgia. Also, wow this post is already 2 years old.
DVDs:
Avengers Assemble
Back to the Future Trilogy
Batman Begins/The Dark Knight
The Dark Knight Rises
Batman: The Movie (1966)
Bean: The Ultimate Disaster Movie
Captain America: The First Avenger
Daredevil
District 9
Doctor Who DVDs (these are in chronological order)
Lost in Time
The Beginning Box Set (An Unearthly Child, The Daleks, The Edge of Destruction)
The Invasion
Peladon Tales
The Three Doctors
The Time Warrior
Genesis of the Daleks
Planet of Evil
The Brain of Morbius
The Robots of Death
The Invasion of Time
Destiny of the Daleks
Earthshock
The Five Doctors
Resurrection of the Daleks
Attack of the Cybermen
Revelation of the Daleks
Rememberance of the Daleks Special Edition
Doctor Who Series One Volume 1
Doctor Who Series One Volume 2
Doctor Who Series One Volume 3
Doctor Who Series One Volume 4
The Complete Second Series
The Complete Third Series
The Complete Fourth Series
The Complete Fifth Series
The Complete Sixth Series
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Elf
E.T. The Extra Terrestial
Family Guy Season One
Family Guy Season Two
Family Guy Season Three
Family Guy: Blue Harvest
Fantastic Four
Fantastic Four: Rise of the Silver Surfer
Finding Nemo
Fonejacker Series 1 and 2 + Facejacker Series 1
Futurama Season 1
Futurama Season 2
Ghostbusters 1 and 2
The Grinch (2000 live action film)
The Incredibles
Indiana Jones: The Complete Collection (Movies 1-4)
Iron Man
Iron Man 2
The IT Crowd Series 1/2
The IT Crowd Series 3
Jason Manford Live at the Manchester Apollo
John Bishop Live
Lee Evans Complete Live Comedy Collection 1994-2005
Little Britain Series 1 - 3 Box Set
Lord of the Rings: Fellowship of the Ring
Lord of the Rings: The Two Towers (Special Extended DVD Edition)
Michael McIntyre 'Hello Wembley!'
The Mighty Boosh Special Edition DVD (Series 1-3)
Monsters, Inc
Monty Python's Flying Circus: The Complete Box Set
Monty Python: The Movies
Mr Bean's Holiday
Night at the Museum
Night at the Museum 2
Nightmare Before Christmas
Outnumbered Series One and Two
Paul
Pirates of the Caribbean Trilogy Box Set
Ramsay's Kitchen Nightmares Revisited
Ratatouille
Russell Howard Live + Live 2: Dingledodies
Sherlock Series One and Two
Shrek
Shrek 2
Spiderman
Spiderman 2
Spiderman 3
Star Wars Episode III: Revenge of the Sith
Star Wars: The Original Trilogy
Stuart Little
Stuart Little 2
The Terminator
Terminator 2: Judgement Day
Terminator 3: Rise of the Machines
Christmas with the Simpsons
The Simpsons Christmas 2
The Simpsons Classics: Bart Wars
The Simpsons Classics: Greatest Hits
The Simpsons Classics: On Your Marks, Get Set, D'oh!
The Simpsons Movie
Transformers (2007)
Transformers: Revenge of the Fallen
Wallace and Gromit - 3 Cracking Adventures
Wall-e
Willy Wonka and the Chocolate Factory
Total: 101